Identification of Abiotic Degradation Pathways of Chlorinated Ethenes by Compound-specific Stable Isotope Analysis: A Proof-of-Concept Study

Abstract

Legacy spills of chlorinated ethenes (CEs) remain one of the key environmental challenges, at DOD facilities and elsewhere, in the US and worldwide. At certain sites, abiotic degradation of CEs may be an important attenuation mechanism. Unequivocal demonstration and quantitation of abiotic contaminant mass destruction remains difficult, typically, due to the absence of pathway-specific degradation products or due to poor mass balance of such products. To fully benefit from abiotic degradation in contaminant remediation work, the process must be documentable. This study explored the utility of multielement Compound-specific Isotope Analysis (CSIA) to identify evidence of abiotic degradation in scenarios with concurrent abiotic and biological degradation. The objective was to identify isotope parameters that would be diagnostic of abiotic pathways including in the present of degradation yield from concurrent biodegradation of the same CEs.

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Document Details

Document Type
Technical Report
Publication Date
Jul 26, 2021
Accession Number
AD1159154

Entities

People

  • Tomasz Kuder

Organizations

  • University of Oklahoma

Tags

Communities of Interest

  • Biomedical

DTIC Thesaurus Topics

  • Alkenes
  • Biodegradation
  • Chemical Kinetics
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Data Sets
  • Department Of Defense
  • Ecology
  • Environment
  • Groundwater
  • High Temperature
  • Hydrogen
  • Isotope Exchange
  • Isotopes
  • Mass Spectrometry
  • Spectrometry

Fields of Study

  • Environmental science

Readers

  • Groundwater Contamination Remediation.
  • Systems Analysis and Design