Protein Sorbents for PFAS-Contaminated Water Treatment: Focused Sorption Kinetics, Protein Degradation, and Thermal Regeneration Testing

Abstract

This project aimed to (1) quantify kinetics of PFAS sorption to select proteins, which is needed to assess viability of protein sorbents to effectively treat AFFF-contaminated groundwater under realistic treatment train conditions, (2) assess protein stability and sorption performance over time under groundwater treatment-relevant conditions, and finally (3) investigate thermal regeneration of the protein sorbents and post-regeneration sorption effectiveness. Detecting and quantifying sorption at low PFAS concentrations during this one year follow-on effort proved challenging, suggesting a pre-concentration step would be needed for current suite of PFAS and proteins tested. Mammalian protein sorbents were not stable under ambient conditions for extended time; microbial- and plant-derived proteins may hold promise. Surface plasmon residence-determined binding kinetics and affinity for PFAS-protein pairs reported herein constitute a significant contribution to science.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Oct 30, 2021
Accession Number
AD1182146

Entities

People

  • C. Heron
  • C. Ng
  • H. Smaili
  • Jeffrey J. Field
  • L. C. Moores
  • M. Michalsen
  • P. U. Fernando

Organizations

  • United States Army Corps of Engineers

Tags

Communities of Interest

  • Biomedical

DTIC Thesaurus Topics

  • Acetic Acid
  • Acids
  • Albumins
  • Availability
  • Carrier Proteins
  • Chemical Synthesis
  • Chemistry
  • Covid-19
  • Department Of Defense
  • Engineers
  • Fatty Acids
  • Graphics Processing Unit
  • Kinetics
  • Liquid Chromatography
  • Mass Spectrometry
  • Proteins
  • Range Finding
  • Surface Plasmon Resonance
  • Surface Plasmons
  • Water
  • Water Purification

Fields of Study

  • Environmental science

Readers

  • Agricultural Chemistry/Soil Science
  • Internal Combustion Engine (ICE) Technology.
  • Molecular and Cellular Biochemistry

Technology Areas

  • Biotechnology
  • Biotechnology - Bioremediation