Developing a MALDI/PET Early Warning Imaging System for Lethal Prostate Cancer

Abstract

Prostate cancer is not only heterogeneous among individuals, but tumors are heterogeneous on the molecular level within a given individual. One well-documented phenomenon is the presence of castrate-resistant prostate cancer with neuroendocrine features (CRPCNE) that evolves over the course of anti-androgen therapy. Our group has discovered that CRPC-NE have a unique cell surface glycan composition enriched with fucose sugars. Therefore, the ability to image glycan fucosylation could be used to predict the emergence of lethal prostate cancer in men. This proposal tests the feasibility of a previously developed PET agent, [18F] fluorofucose (Fuc-PET) as afunctional method to quantify PCa glycan fucosylation, and thus, the burden of lethal disease using animal models. Our hypothesis is that Fuc-PET can quantify the amount of glycan fucosylation in tumors noninvasively and thus predict aggressive pathology in vivo.Thus far,we have discovered significant advancements in the field. First, we discovered a fucosylated glycan signature that predicts the development of metastatic prostate cancer at the time of prostatectomy. Second, small molecule inhibition of glucose metabolism and fucosylation has a supportive effect on tumor growth because of immune system inhibition. We have overcome that limitation with the ketogenic diet. These findings indicate that dietary modifications could enhance therapeutic efficacy in men with advanced prostate cancer.

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Document Details

Document Type
Technical Report
Publication Date
Oct 01, 2022
Accession Number
AD1201598

Entities

People

  • Joseph Ippolito

Organizations

  • Medical University of South Carolina
  • Northwestern University
  • Washington University in St. Louis

Tags

DTIC Thesaurus Topics

  • Androgen Receptors
  • Androgens
  • Biomedical Research
  • Cancer
  • Carbohydrates
  • Cells
  • Chemistry
  • Culture Techniques
  • Diseases
  • Immune System
  • Immunotherapy
  • Inhibition
  • Lung Cancer
  • Lymphocytes
  • Mass Spectrometry
  • Molecules
  • Neoplasms
  • Prostate Cancer
  • Proteins
  • Therapy
  • Tissues

Fields of Study

  • Biology
  • Physics

Readers

  • Immunology
  • Oncology
  • Prostate Cancer Biology.