Development of Novel Functionalized Polymeric Thin Films for Equilibrium Passive Sampling of PFAS in Surface and Groundwater

Abstract

The overarching goal of this 1-year SERDP SEED project was to develop and test a range of functionalized polymeric membranes for use in equilibrium passive sampling of PFAS compounds. The following objectives were addressed in this project: 1) develop novel polymeric thin films for equilibrium passive sampling that will be either solid or liquid sorbents embedded in a thin polymer sheet; 2) perform equilibrium partitioning studies with PFAS compounds covering a range of properties and interpret isotherm data based on sorption models; 3) test equilibrium reversibility for the top two choices of polymers and assess the use of performance reference compounds to quantify the extent of equilibrium; 4) evaluate the mechanism of the sorption process. We demonstrate that several composite polymers can be synthesized that remain stable in the water environment and provide adequate sorption of PFAS from aqueous solution at equilibrium. Initial results presented in this report show great promise for pursuing the concept of equilibrium passive sampling for PFAS in water.

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Document Details

Document Type
Technical Report
Publication Date
Apr 01, 2022
Accession Number
AD1202905

Entities

People

  • Batool Murtadha
  • Gregory Foster
  • Matthew Badia
  • Songjing Yan
  • Upal Ghosh

Organizations

  • George Mason University
  • University of Maryland, Baltimore County

Tags

Communities of Interest

  • Advanced Electronics
  • C4I
  • Ground and Sea Platforms

DTIC Thesaurus Topics

  • Chemical Synthesis
  • Chemistry
  • Ecology
  • Ecotoxicology
  • Environmental Protection
  • Fatty Acids
  • Liquid Chromatography
  • Mass Spectrometry
  • Mass Transfer
  • Materials Laboratories
  • Materials Science
  • Measurement
  • Metallic Nanoparticles
  • Organic Chemistry
  • Organic Compounds
  • Polymer Chemistry
  • Polymeric Films

Readers

  • Agricultural Chemistry/Soil Science
  • Fire Suppression Systems Design.
  • Nanocomposite Materials Science