Application of Carbon and Nitrogen Stable Isotope Analysis to Evaluate Biotic and Abiotic Degradation of DNAN and NTO

Abstract

The key objectives of this project were (1) to develop and validate compound-specific stable isotope analysis (CSIA) methods for carbon and nitrogen in the insensitive munitions constituents 2, 4-dinitroanisole (DNAN) and 3-nitro-1, 2, 4-triazol-5-one (NTO) and (2) to quantify kinetic isotope effects in carbon and nitrogen during the biotic and abiotic degradation of these compounds. These objectives were accomplished. The resulting isotopic enrichment parameters provide insights into natural and engineered degradation pathways and new diagnostic measurement tools that will allow the extent of in situ degradation to be quantified in soils and natural waters on ranges and other contaminated sites. This research was responsive to ERSON-17-03 as it provides new methods to "develop an improved understanding of the fate and effects of the components DNAN and NTO that are used in the insensitive munitions formulations." This project also provides a valuable means by which to assess the necessity and effectiveness of in situ enhancement of biotic and/or abiotic degradation strategies for these insensitive munitions compounds.

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Document Details

Document Type
Technical Report
Publication Date
Sep 22, 2022
Accession Number
AD1206361

Entities

People

  • Chunlei Wang
  • Linnea J. Heraty
  • Mark E. Fuller
  • Neil C. Sturchio
  • Paul B. Hatzinger

Organizations

  • University of Delaware

Tags

Communities of Interest

  • Biomedical
  • Energy and Power Technologies
  • Space
  • Weapons Technologies

DTIC Thesaurus Topics

  • Chemical Analysis
  • Chemical Engineering
  • Chemical Reactants
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Environmental Restoration And Remediation
  • Fungi
  • Insensitive Explosives
  • Isotopes
  • Liquid Chromatography
  • Mass Spectrometry
  • Materials Laboratories
  • Materials Processing
  • Materials Science
  • Nitrogen Oxides
  • Organic Chemistry

Fields of Study

  • Environmental science

Readers

  • Agricultural Chemistry/Soil Science
  • Groundwater Contamination Remediation.
  • Systems Analysis and Design