Optimized Reduced Spectrum Models of Diffuse Reflectance for NIR-SWIR Absorbing-Dye Formulations

Abstract

This study describes a measurement-optimized parametric model of diffuse reflectance, based on the reduction of absorption spectra for Near Infrared (NIR) and Short-Wave Infrared (SWIR) absorbing dyes on substrates using critical feature isolation and projection. The critical features are identified through a structural analysis of the peaks, troughs, and points of inflection within the Kubelka-Munk absorption spectra, which is calculated from diffuse reflectance measurements. These critical features are then parameterized and projected into a reduced feature subspace using Lorentzian decompositions to effectively capture the fundamental characteristics of the absorbing dyes, while removing processing and measurement noise. A Kramers-Kronig analysis then characterizes the dielectric responses and provides an estimation of the reduced spectra reflectance. The model parameters for the analytical reduction are further refined using a nonlinear multivariable optimization function between the analytically predicted reflectance and the measured reflectance. This results in an enhanced measurement-optimized model that is capable of incorporating measurement and processing artifacts to improve application-specific reflectance predictions. Furthermore, the reduced, enhanced functions establish a parametric dataspace that can support the mapping of functions between individual NIR-SWIR absorbing dye components and the diffuse reflectance predictions for new mixture and substrate combinations.

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Document Details

Document Type
Technical Report
Publication Date
Nov 09, 2023
Accession Number
AD1214951

Entities

People

  • Rachel Viger
  • Samuel G. Lambrakos
  • Scott A. Ramsey
  • Troy Mayo

Organizations

  • United States Naval Research Laboratory

Tags

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Artifacts
  • Materials
  • Measurement
  • Military Research
  • Optical Phenomena
  • Optical Properties
  • Optimization
  • Reflectance
  • Refraction
  • Refractive Index
  • Scattering
  • Short-Wavelength Infrared Radiation
  • Spectra
  • Structural Analysis
  • Substrates

Readers

  • Approximation Theory.
  • Ocean-Atmosphere Mesoscale Modeling, Data Assimilation, and Flux Boundary Layers
  • Spectroscopy.