Thermal Destruction of PFAS by Hydrodynamic Cavitation

Abstract

Per- and polyfluoroalkyl substance (PFAS) contamination of groundwater is pernicious and widespread, potentially contaminating the drinking water of millions of Americans. A major source of this contamination is aqueous film forming foam which was used for decades for firefighting and is still in use today . The Department of Defense has identified hundreds of military sites where water has been contaminated by PFAS and a full DoD clean-up effort is expected to cost billions of dollars. Existing options to destroy PFAS are limited and expensive. We have demonstrated a novel technique for thermal destruction of PFAS. The low-cost process uses hydrodynamic cavitation (HC) to thermally destroy PFAS in water. We optimized flow parameters using methylene blue dye to measure oxidation rates across a wide range of conditions. We then demonstrated destruction of perfluorooctanesulfonic acid (PFOS) by HC in a series of tests that show the effects of reactor design and operating conditions. We measured the rates of PFOS destruction as well as concentration of reaction products as a function of time after starting the process. We found that HC was a robust process that effectively destroyed PFAS across the range of conditions tested.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 2023
Accession Number
AD1216385

Entities

People

  • Anthony Bednar
  • Gabrielle David
  • Michael Izenson
  • Rachel Gilmore

Organizations

  • Creare, Inc.
  • Engineer Research and Development Center

Tags

DTIC Thesaurus Topics

  • Chemical Engineering
  • Chemical Synthesis
  • Chemistry
  • Computational Science
  • Ecology
  • Electrospray Ionization
  • Environment
  • Environmental Protection
  • Environmental Restoration And Remediation
  • Fluorinated Hydrocarbons
  • Groundwater
  • Liquid Chromatography
  • Mass Spectrometry
  • Measurement
  • Organic Chemistry
  • Test Facilities
  • Water Purification

Fields of Study

  • Environmental science

Readers

  • Educational Psychology
  • Fire Suppression Systems Design.
  • Organic Chemistry