An EMF Method for the Determination of Transference Numbers in Molten Salt Mixtures.

Abstract

Transference numbers of the cations relative to the chloride ion in molten mixtures of alkali chloride - cerium chloride were determined from emf measurements on concentration cells with transference of the type: (-)H2, HCl(g)-C/MCl/Al203/MCl,CeCl3/C-HCl,H2(g)(+), where M is Li, Na, or K. The cells were operated with a mixture of hydrogen and hydrogen chloride gases instead of chlorine gas to minimize the possibility, if any, of the oxidation of cerous chloride to ceric chloride. The emf measurements were carried out at 850C and results are presented over the entire composition range of the systems studied. It was also shown that, in these mixtures, the alkali ions possess a relatively larger mobility than the cerous ion.

Document Details

Document Type
Technical Report
Publication Date
Oct 01, 1974
Accession Number
ADA001528

Entities

People

  • Wishvender K. Behl

Organizations

  • United States Army Communications-Electronics Command

Tags

DTIC Thesaurus Topics

  • Chlorides
  • Chlorine
  • Chlorine Compounds
  • Elements
  • Halogen Compounds
  • Halogens
  • Hydrogen
  • Measurement
  • Mobility
  • Oxidation

Readers

  • Analytical Chemistry
  • Materials Science and Engineering.