Effect of Selected Impurities on the High Temperature Mechanical Properties of Hot-Pressed Silicon Nitride

Abstract

The strength of commercial hot-pressed silicon nitride has been shown to degrade severely at elevated temperatures. As the temperature is increased the amount of non-elastic deformation occurring prior to fracture has been found to increase significantly. This reduction in high temperature strength and creep resistance is believed to be associated with impurities. Selected impurities were therefore added as oxides or carbonates (Al2O3, CaO, Fe2O3, Li2CO3 and Na2CO3) to both a relatively pure alpha-phase silicon nitride powder and a relatively pure beta-phase silicon nitride starting powder. These powders were then hot-pressed to full density using 5 wt % MgO as the pressing additive. The silicon nitride hot-pressed from the alpha-phase powder exhibits higher strength at both 25C and 1400C than that fabricated from the beta-phase powder. The impurity additions had no effect on the room temperature mechanical properties.

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Document Details

Document Type
Technical Report
Publication Date
Oct 18, 1974
Accession Number
ADA002251

Entities

People

  • E. S. Diaz
  • F. F. Lange
  • J. L. Iskoe

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Additives (Chemicals)
  • Beta Testing
  • Boundaries
  • Carbonates
  • Ceramic Materials
  • Contracts
  • Creep
  • Creep Tests
  • Deflection
  • Flexural Strength
  • Grain Boundaries
  • High Temperature
  • Hot Pressing
  • Impurities
  • Materials
  • Mechanical Properties
  • Resistance

Fields of Study

  • Materials science

Readers

  • Powder metallurgy of Titanium alloys.