Dynamic Mechanical and Morphological Studies of Homopolymer/Block Copolymer Blends.

Abstract

A triblock copolymer of styrene-butadiene-styrene (SBS) was blended with a high and a low molecular weight polybutadiene (designated as PB(H) and PB(L) respectively). Electron micrographs of these blends show that PB(L) was solubilized into the butadiene domains of the SBS; while PB(H) was present in a separate phase. Dynamic mechanical data of the SBS/PB(L) blends indicate the presence of an intermediate loss peak between those of the glass transitions of the styrene and butadiene blocks in SBS, which can be attributed to the slippage of untrapped entanglements of PB(L) chains. Similar data for blends containing PB(H) also shows an intermediate loss peak, which is, however, due to crystallization and melting of the poly-cis-butadiene chains. Dynamic mechanical data for crosslinked blends were also taken for comparison.

Document Details

Document Type
Technical Report
Publication Date
Jan 15, 1975
Accession Number
ADA004643

Entities

People

  • L. Toy
  • M. Niinomi
  • Meikun Shen

Organizations

  • University of California, Berkeley

Tags

DTIC Thesaurus Topics

  • Alkenes
  • Block Copolymers
  • Butadienes
  • Copolymers
  • Crystallization
  • Electrons
  • Macromolecules
  • Molecular Weight
  • Molecules
  • Polybutadiene
  • Polymers
  • Synthetic Rubber
  • Transitions

Fields of Study

  • Materials science

Readers

  • Polymer Science and Technology

Technology Areas

  • Microelectronics