Preparation and Properties of eta 6-Tricarbonylchromium - Complexed Arylenesiloxane Polymers.

Abstract

Poly(tetramethyl-p-silphenylenesiloxane), 1, and poly(methylphenylsiloxane), 2, were prepared and subsequently reacted with hexacarbonylchromium to generate their eta 6-Cr(CO)3 complexed analogs 3 and 4 respectively. During the complexation reaction, competing decomposition to chromium salts took place. Furthermore a competing chain scission reaction took place resulting in lower molecular weights for the complexed polymers. Heating 3 and 4 resulted in carbon monoxide evolution and the presence of eta 6-Cr(CO)3 moieties lowered the thermal stability of the polymers.

Document Details

Document Type
Technical Report
Publication Date
Jan 15, 1975
Accession Number
ADA004951

Entities

People

  • Charles U. Pittman Jr.
  • Samuel P. Mcmanus
  • William J. Patterson

Organizations

  • University of Alabama

Tags

DTIC Thesaurus Topics

  • Carbon Monoxide
  • Chemical Compounds
  • Chromium
  • Decomposition
  • Dielectric Gases
  • Dielectrics
  • Fluids
  • Gases
  • Materials
  • Molecular Weight
  • Monoxides
  • Personal Information Managers
  • Thermal Stability

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry
  • Polymer Science and Technology