Lithium-Inorganic Electrolyte Batteries.

Abstract

An all-inorganic electrolyte, lithium primary battery operable over the temperature range -40 to +160F is being evaluated. The desired energy density is 150 watt-hours per pound of total battery weight and the desired power density is 50 watts per pound. Sulfur is a reaction product of Li/SOCl2 cells. Fifty percent (50%) of the total sulfur content of reacted SOCl2 is found by chemical analysis of elemental sulfur. Sulfur is quite soluble in the electrolyte. Analysis by gas chromatography indicates that SO2 is a reaction product, but no other major volatile products are formed. Reduction of SOCl2 on Ni, Pt, Au and C is a complex, potential dependent process. Surface layers are formed on all these electrodes and interfere with reduction of SOCl2. After high temperature storage, Li/SOCl2 batteries showed severe voltage delays and voltage depression due to Li electrode polarization. The protective film on Li breaks only locally leading to localized anodic Li dissolution at high current densities.

Document Details

Document Type
Technical Report
Publication Date
Apr 01, 1975
Accession Number
ADA009782

Entities

People

  • David E. Toland
  • Gerhard L. Holleck
  • Michael J. Turchan

Tags

Communities of Interest

  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Analytical Chemistry Techniques
  • Chemical Analysis
  • Chromatography
  • Current Density
  • Depression
  • Electrodes
  • Electrolytes
  • Energy
  • Gas Chromatography
  • High Temperature
  • Polarization
  • Primary Batteries
  • Storage

Fields of Study

  • Materials science

Readers

  • Analytical Chemistry
  • Battery Technology and Engineering
  • Surface Engineering/Surface Coating Technology.