The Heterogeneous Decomposition of Hydrazine. Part 6. Kinetics of the Decomposition on Supported Palladium and Platinum Catalysts

Abstract

The decomposition of hydrazine on either a palladium or a platinum catalyst may be represented by the reaction 2N2H4 to N2 +H2 + 2NH3. The observed one half order kinetics, changing to zero order with platinum, may be explained by deriving rate equations from the Langmuir adsorption isotherm and assuming that the initial, slow, step is the dissociative chemisorption of hydrazine in the form of NH2 radicals. In accordance with the dual plane theory of Cosser and Tompkins it is suggested that the adsorption process and subsequent reaction occur only on the active sites of these metals. Because these catalysts are much less active than a supported iridium catalyst neither is considered as an alternative for use in catalytic hydrazine thrusters.

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Document Details

Document Type
Technical Report
Publication Date
Nov 01, 1974
Accession Number
ADA013003

Entities

People

  • C. F. Sayer

Tags

Communities of Interest

  • Air Platforms
  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Adsorption
  • Catalysts
  • Chemical Reactions
  • Chemisorption
  • Decomposition
  • Determinants (Mathematics)
  • Energy
  • Equations
  • Experimental Data
  • Foreign Languages
  • Gas Chromatography
  • Heat Of Activation
  • Hydrazines
  • Isotherms
  • Metals
  • Nitrogen Compounds
  • Reaction Mechanisms

Fields of Study

  • Chemistry

Readers

  • Combustion science or combustion engineering.
  • Quantum Chemistry
  • Surface Engineering/Surface Coating Technology.

Technology Areas

  • Space
  • Space - Hall-Effect Thruster