Water Proton Relaxation as a Monitor of Membrane-Bound Manganese in Spinach Chloroplasts.

Abstract

First measurements of proton relaxation on chloroplast membranes are presented here. Experiments show that the water proton spin-lattice relaxation rate in chloroplast thylakoid membrane suspensions can be used to monitor membrane-bound manganese. The relaxation effect is reduced to 0.4 of its original value upon manganese extraction by washing with either alkaline tris buffer of NH2OH-EDTA solution. Large increases in the proton relaxation rate are measured in the presence of reductants such as tetraphenylboron and NH2Oh; oxidants such as potassium ferricyanide or 2,6-dichlorophenolindophenol lead to a decrease in this rate. These results suggest that manganese exists as a mixture of oxidation states in dark-adapted chloroplasts.

Document Details

Document Type
Technical Report
Publication Date
Oct 03, 1975
Accession Number
ADA016646

Entities

People

  • Govindjee
  • N. Zumbulyadis
  • P. G. Schmidt
  • T. Wydrzynski

Organizations

  • University of Illinois Urbana–Champaign

Tags

DTIC Thesaurus Topics

  • Anatomy
  • Biological Sciences
  • Cyanides
  • Elements
  • Extraction
  • Manganese
  • Measurement
  • Membranes
  • Metals
  • Oxidation
  • Plastids
  • Potassium

Readers

  • Analytical Chemistry
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Molecular and Cellular Biochemistry