Coulombic Capacities of Carbon Cathodes in Lithium-Thionyl Chloride Cells.

Abstract

For lithium-thionyl chloride cells utilizing Teflon-bonded carbon cathodes, the attainable energy decreases with decreasing temperature and increasing rate of discharge. The losses correspond largely to decreases in the apparent coulombic capacities of the cathodes. The cathode capacity appears to depend directly on the overall porosity of the electrode rather than on the surface area of the carbon. At room temperature, cathode end-of-life occurs when the clogging of pores with product lithium chloride causes a sharp rise in concentration polarization. The clogging of cathode pores occurs earlier at low temperature, likely due to the precipitation of another reaction product, perhaps sulfur. (Author)

Document Details

Document Type
Technical Report
Publication Date
Nov 01, 1975
Accession Number
ADA018024

Entities

People

  • John A. Christopulos
  • Sol Gilman

Organizations

  • United States Army Communications-Electronics Command

Tags

DTIC Thesaurus Topics

  • Chlorides
  • Electrodes
  • Low Temperature
  • Polarization
  • Porosity
  • Precipitation

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies