Microheterogeneity and Structure Formation in Amorphous Polyurethane Block Copolymers (O Yavleniyakh Mikrogeterogennosti i Strukturoobrazovaniya v Amorfnykh Poluretanovykh Blok-Sopolimerakh),

Abstract

The authors have shown in their earlier work (1) that crystallization of at least one block components of a copolymer changes some properties of the whole copolymer. For example, the glass transition temperature (Tc) of one component could decrease in the course of crystallization the Tc of another component which is characterized by much lower Tc. The observed phenomenon was explained by a concentration of homogeneous blocks in microvolumes, i.e., an appearance of the microheterogeneity in block copolymers during crystallization. A division of the block copolymer components into microregions was also observed among amorphous copolymers, with components markedly different with respect to polarity (2). It could be expected that appearance and development of the microheterogeneity in similar systems would produce characteristic changes in thermomechanical properties. In this work amorphous block copolymers consisting of poly(ethylene adipate) and poly(propylene phthalate), crosslinked with OCN(CH2)6NCO.

Document Details

Document Type
Technical Report
Publication Date
Feb 04, 1976
Accession Number
ADA021185

Entities

People

  • A. G. Sinaiskii
  • B. Ya. Teitelbaum
  • E. G. Gubanov

Organizations

  • Office of Naval Intelligence

Tags

DTIC Thesaurus Topics

  • Alkenes
  • Block Copolymers
  • Copolymers
  • Crystallization
  • Ethylenes
  • Glass Transition Temperature
  • Phase Transformations
  • Propenes
  • Transition Temperature
  • Transitions

Readers

  • Materials Science and Engineering.
  • Polymer Science and Technology

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene