Macromolecular Characterization of Poly(bis(M-Chlorophenoxy)-Phosphazene)

Abstract

The macromolecular structures and structure-property relationships of five poly(bis(m-chlorophenoxy)phosphazene) samples are critically analyzed. The polymers are found to have high molecular weights and broad, bimodal molecular weight distributions. Differences are observed in polymer chain structure (branching) and solubility characteristics. An intrinsic viscosity-molecular weight relationship is established for the linear polymer in chloroform solution at 25C. The rate and mechanism for the thermal degradation in air of the polyphosphazenes are investigated and compared with that of polystyrene. Mechanical properties, thermal transitions, and thermal stability are markedly influenced by differences in the macromolecular and chemical structures of the polymers.

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Document Details

Document Type
Technical Report
Publication Date
Aug 01, 1976
Accession Number
ADA032039

Entities

People

  • Bernard R. Laliberte
  • Elizabeth R. Plumer
  • Gary L. Hagnauer
  • Robert E. Singler
  • Susan J. Kalian

Organizations

  • United States Army Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Space
  • Weapons Technologies

DTIC Thesaurus Topics

  • Chemistry
  • Crystal Lattices
  • Dielectric Polymers
  • Glass
  • Glass Transition Temperature
  • Materials
  • Materials Laboratories
  • Mechanical Properties
  • Mechanics
  • Military Research
  • Molecules
  • Polymer Chemistry
  • Polymeric Films
  • Polymers
  • Thermal Stability
  • Transition Temperature
  • Viscosity

Fields of Study

  • Chemistry

Readers

  • Polymer Science and Technology