The Adsorption of Chromium (VI) at the Oxide/Water Interface

Abstract

Because of its toxicity, chromium has a potential environmental impact, and it is imperative that mechanisms which control the movement of this metal through the environment be known. It has been documented that adsorption to suspended and deposited materials is important in controlling the concentration of heavy metals in natural waters. Numerous previous investigations have been concerned with the adsorption of hydrolyzable heavy metals; however, chromium exists in aqueous solution as the anionic oxocomplex. In this report data on adsorption of chromium and phosphate are compared at the water interface of various metal oxides. The conclusions of this investigation are: (1) for Al2O3 both chromium and phosphate adsorb at low pH's; however, upon increasing pH, there is a decrease in the percentage adsorption; (2) chromium adsorption decreases with increasing ionic strength; (3) phosphate exhibits a higher specific adsorption energy than does chromium; (4) adsorption of both chromium and phosphate is low for solids which have isoelectric points at low pH's; (5) with a more valid method of determining the surface potential other than the Nernst equation, the simple electrical double layer model can be used to give reasonable predictions of the pH and surface charge response for adsorption of anions.

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Document Details

Document Type
Technical Report
Publication Date
Sep 01, 1975
Accession Number
ADA032083

Entities

People

  • Michael G. Macnaughton

Tags

Communities of Interest

  • Air Platforms
  • Biomedical

DTIC Thesaurus Topics

  • Adsorption
  • Air Force
  • Aluminum Oxides
  • Aqueous Solutions
  • Chemical Synthesis
  • Chemistry
  • Chromium Compounds
  • Civil Engineering
  • Engineering
  • Environment
  • Equations
  • Heavy Metals
  • Metal Oxides
  • Oxidation
  • Oxides
  • Physical Chemistry
  • Water

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Surface Engineering/Surface Coating Technology.
  • Theoretical Analysis.