Antiwear Additives, Wear Studies on Chemical Addition Agents for Imparting an Effective Lubricating Response in Polysiloxane (Silicone) Fluids

Abstract

An additive package based on chlorendate and thiadiazole molecular structures has been discovered which imparts antiwear properties to tetrachlorophenylmethyl siloxane fluids that have been previously unattainable. For the first time a polysiloxane based fluid possessing antiwear properties comparable to such outstanding lubricants as petroleum oils, synthetic hydrocarbons, diesters and phosphate esters was formulated. In addition, a detailed analysis of the modification of friction surfaces (steel-on-steel) using organophosphate addition agents in polysiloxane fluids has refuted the commonly held belief that the inability of antiwear additives to function in polysiloxane media at low concentrations is due to the fact that the additive is substantially excluded from the surface. Evidence is presented to show that additive-surface interactions are indeed prevalent resulting in an antagonistic (pro-wear) action. In one specific instance depending on load and concentration a beneficial lubricating response is achieved with a tetrachlorophenylmethyl siloxane fluid containing alkyl-phosphate derivatives. The use of organo- phosphates as antiwear agents in polysiloxane has previously proved unfruitful, therefore, these results represent a significant area for further study.

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Document Details

Document Type
Technical Report
Publication Date
Jul 02, 1976
Accession Number
ADA033527

Entities

People

  • Alfeo A. Conte Jr.
  • James L. Hammond

Organizations

  • Naval Air Warfare Center Warminster

Tags

Communities of Interest

  • Advanced Electronics
  • Air Platforms

DTIC Thesaurus Topics

  • Aircrafts
  • Chemical Compounds
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Films
  • Friction
  • Hydrocarbons
  • Lubricants
  • Lubrication
  • Materials
  • Metals
  • Military Aircraft
  • Organic Compounds
  • Organophosphates
  • Polymers
  • Surface Chemistry

Readers

  • Petroleum Engineering
  • Polymer Science and Engineering.
  • Theoretical Analysis.