Sealed Primary Lithium-Inorganic Electrolyte Cell.

Abstract

The Li/SOCl2 hermetic D cell developed by P. R. Mallory and Co. Inc. met or exceeded all the initial objectives such as E. D. of 150 WHr/lb at thrity hours rate and a peak power density of 50 watts/lb and the storage and operating temperature of -40 to 160 C. The two major deficiencies exhibited by the cells were explosion hazard on abuse and voltage delay on storage. Both the problems were studied in detail and considerable progress has been made in both the above areas. During the last quarter, we continued the SEM studies of the Li that was found to be responsible for the voltage delay. We obtained LiCl film growth rate curves for the Li samples stored in the electrolytes containing various salt concentrations and additives at 72, 55 and 25 C. We found that the growth rates were substantially reduced by reducing the salt concentration. Also the addition of SO2 caused the LiCl film to grow in a more orderly fashion. We plan to examine the effect of these electrolyte variables on the voltage delay of the practical hermetic Li/SOCl2D cells during the next quarter. We have set up a DTA apparatus for doing differential thermal analysis of the various chemicals present in a fresh and/or partially discharged Li/SOCl2D cell. Preliminary data obtained so far indicate that it is possible to distinguish between pressure bursts and a thermal runaway by this method.

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Document Details

Document Type
Technical Report
Publication Date
Dec 01, 1976
Accession Number
ADA034069

Entities

People

  • A. N. Dey

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Chemical Compounds
  • Chemical Reactions
  • Chemistry
  • Crystals
  • Differential Thermal Analysis
  • Electrochemical Reactions
  • Electrolytes
  • Electron Microscopes
  • Electronics Laboratories
  • Energy
  • Energy Storage
  • Epitaxial Growth
  • Films
  • Measurement
  • Melting Point
  • Storage
  • Thermal Analysis

Fields of Study

  • Materials science

Readers

  • Battery Technology and Engineering
  • Systems Analysis and Design
  • Thin Film Deposition Science.