Photoisomerization of Linked Anthracenses. A Demanding Test of Molecular Geometry for Intermediates in Photodimerization.

Abstract

Valence photoisomerization and photophysical properties of a series of dianthry-lethanes, dianthrylmethanes, and tetrabenzo(2.2)paracyclophane are reported. Fluorescence lifetimes and quantum yields depend upon the nature of the linkage between anthracene moieties. Quantum efficiency for photoisomerization depends on the substitution pattern at 10,10 prime positions. Sandwich dimers with excimer-like interaction are generated on low temperature photolysis in glasses of dianthrylethane but not dianthrylmethane. It is concluded that geometrical requirements for excimerization and photodimerization are quite different. (Author)

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Document Details

Document Type
Technical Report
Publication Date
Dec 01, 1976
Accession Number
ADA034176

Entities

People

  • Guilford Jones Ii
  • William R. Bergmark

Organizations

  • Boston University

Tags

Communities of Interest

  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Absorption Spectra
  • Aromatic Polycyclic Hydrocarbons
  • Chemistry
  • Efficiency
  • Emission
  • Fluorescence
  • Geometry
  • Low Temperature
  • Massachusetts
  • Military Research
  • New York
  • Photolysis
  • Quantum Efficiency
  • Quantum Yields
  • United States
  • United States Government
  • Universities

Fields of Study

  • Chemistry

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Theoretical Analysis.

Technology Areas

  • Quantum Computing