Deuterium Exchange at Terminal Boron-Hydrogen Bonds Catalyzed by Certain Transition Metal Complexes. A Qualitative Study of Selectivity and Mechanism.

Abstract

A wide variety of substrates, including carboranes, metallocarboranes, and boron hydrides, were found to undergo catalytic isotopic exchange of terminal hydrogen with deuterium gas in the presence of various transition metal complexes. A mechanism is postulated which rationalizes the varied results and which involves oxidative addition of boron-hydrogen bonds to catalytic species.

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Document Details

Document Type
Technical Report
Publication Date
Mar 15, 1977
Accession Number
ADA038118

Entities

People

  • Elvin L. Hoel
  • M. Frederick Hawthorne
  • Mehdi Talebinasab-savari

Organizations

  • University of California, Los Angeles

Tags

Communities of Interest

  • Air Platforms
  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Alkanes
  • Chemical Products
  • Chemical Reaction Properties
  • Chemical Synthesis
  • Chemistry
  • Coordination Complexes
  • Exchange Reactions
  • Hydrogen
  • Hydrogen Bonds
  • Mass Spectra
  • Mass Spectroscopy
  • Military Research
  • Navy
  • Plastic Explosives
  • Resonance
  • Spectra
  • Spectroscopy

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry