Crystal Structure and Magnetic Studies of Bis (mu-Dibutylphosphinato) Copper (II).

Abstract

The structure of Cu(OP(C4H9)2O)2 in the solid state has been determined by three-dimensional single-crystal x-ray techniques. The structure was solved by the heavy-atom technique, and least squares refinement gave an R factor of 0.061. The structure consists of polymeric chains of copper atoms linked by double phosphinate bridges. The coordination around each copper atom can be described as a very flattened tetrahedron. The g tensors for oriented single crystals were determined by ESR and range from 2.07 to 2.41, with the larger value in a direction nearly normal to a mean plane formed by the copper atoms and the ligands. The spin orbit coupling constant suggests considerable mixing of metal and ligand orbitals in this polymer.

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1977
Accession Number
ADA041510

Entities

People

  • L. S. Smith
  • P. Colamarino
  • P. L. Orioli
  • Paul Newman
  • R. Cini

Tags

Communities of Interest

  • Air Platforms
  • Weapons Technologies

DTIC Thesaurus Topics

  • Chemistry
  • Crystal Structure
  • Crystals
  • Electron Paramagnetic Resonance
  • Electron Spin Resonance
  • Electrons
  • Magnetic Fields
  • Magnetic Properties
  • Materials
  • Metals
  • Military Research
  • New York
  • Orientation (Direction)
  • Paramagnetic Resonance
  • Resonance
  • Rotation
  • Single Crystals

Fields of Study

  • Chemistry

Readers

  • Materials Science and Engineering.
  • Organic Chemistry
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Space