Multimode Modeling of the Water Molecule.
Abstract
This report presents three approaches to multimode modeling water vapor. These are (1) A correlated bender approach that treats fluctuations in the bend angle as well as correlations of the bending mode with the OH stretch mode. Only a single effective nuclear coordinate is used. (2) A model that treats all three vibrational degrees of freedom, mode-mode coupling as well as molecular rotation. In addition, the effects of centrifugal distortion are included in a nonperturbative manner. (3) A phenomenological approach based on the concept of fitting the A, B and C rotation matrices, both diagonal components, to the rotation-vibration energy levels. This approach, although phenomenological in nature is predictive.
Document Details
- Document Type
- Technical Report
- Publication Date
- Aug 01, 1977
- Accession Number
- ADA047397
Entities
People
- D. Rogovin
- T. Stephens
- W. Wilson