Characterization and Continuous Extrusion of Isotropic and Anisotropic Poly(p-Phenylene Terephthalamide)/Sulfuric Acid Solutions to Form Ribbons and Blown Film.

Abstract

An experimental characterization and processing study of redissolved Kevlar and poly(p-phenylene terephthalamide)/sulfuric acid solutions is reported. Polarized light microscopy studies show the development of an anisotropic phase. When two phases coexist, negatively birefringent spherulites are observed. At higher concentrations, a single phase of coalescing spherulites is seen and following melting and subsequent cooling, nematic (threadlike) structures are observed. Viscosity and normal stresses were measured at various concentrations and temperatures. A yield stress is exhibited at room temperature. Both room temperature and 60 degree C viscosity versus concentration curves display maxima. The solutions in concentration ranges from 2 to 12% have been extruded as ribbons and as annular blown tubular film. Processing variables and problems are discussed. Wide angle x-ray scattering patterns of films show orientation. Tensile properties have been measured on films. (Author)

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Document Details

Document Type
Technical Report
Publication Date
Nov 10, 1978
Accession Number
ADA061783

Entities

People

  • Hiroshi Aoki
  • James L. White
  • John F. Fellers
  • Yoshihiko Onogi

Organizations

  • University of Tennessee system

Tags

Communities of Interest

  • Air Platforms

DTIC Thesaurus Topics

  • Air Gaps
  • Aspect Ratio
  • Crystal Structure
  • Diffraction
  • Distortion
  • Films
  • Liquid Crystals
  • Materials
  • Measurement
  • Microscopy
  • Polymers
  • Scattering
  • Spectra
  • Stresses
  • Tensile Strength
  • Viscosity
  • X Rays

Readers

  • Mechanical Engineering/Mechanics of Materials.
  • Polymer Science and Engineering.
  • Polymer Science and Technology