Time-Temperature Studies of High Temperature Deterioration Phenomenon in Lubricant Systems: Synthetic Ester Lubricants.

Abstract

A study of the lengths of the inhibition periods caused by the addition of varying amounts of the bisphenol antioxidant, 4,4'-methylenebis (2,6-di-tertbutylphenol), BPH, on the autoxidation of pentaerythrityl tetraheptanoate, PETH, in a batch reactor at 180, 200 and 220C has been carried out. A kinetic analysis based upon these results together with preliminary results on the BPH decay and quinone methide product formation as a function of time yield a general equation for the rate of decay of BPH. A study of wear rates at 100C manifested by pure PETH and by slightly oxidized PETH has been completed. At one ca. 2% oxidation the wear rate is increased by a factor of 8 over that of pure PETH. This result together with those from various ancillary studies are consistent with the view that hydroperoxides, perhaps in combination with alpha,gamma-substituted difunctional oxidation products, lead to a rapid corrosive wear phenomena. (Author)

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Document Details

Document Type
Technical Report
Publication Date
Oct 01, 1978
Accession Number
ADA064563

Entities

People

  • E. J. Hamilton
  • L. R. Mahoney
  • P. A. Willermet
  • R. K. Jensen
  • S. Korcek

Organizations

  • Ford Motor Company

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Air Force
  • Batch Reactors
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Chromatographic Analysis
  • Contracts
  • Engineering
  • Equations
  • Free Radicals
  • High Temperature
  • Hydrocarbons
  • Inhibition
  • Liquid Chromatography
  • Lubricants
  • Materials
  • Oxidation

Readers

  • Organic Chemistry
  • Petroleum Engineering