Development of Practical MO Techniques for Prediction of the Properties and Behavior of Materials.
Abstract
A new semiempirical method (MNDO), based on NDDO, has proved superior to MINDO/3 in nearly all respects. Parameters are available for H, Be, B, C, N, O, F, and (without 3d AOs) Si, P, S, and C1. MINDO/3 and MNDO give good estimates of molecular vibration frequencies and isotopic shifts, and hence of entropies, specific heats, entropies of activation, and kinetic isotope effects. MNDO calculations were carried out for a number of normal and mesoionic oxazoles and imidazoles and for pentadienyl ions and their methyl derivatives. (Author)
Document Details
- Document Type
- Technical Report
- Publication Date
- Oct 31, 1978
- Accession Number
- ADA067068
Entities
People
- Michael J. S. Dewar
Organizations
- University of Texas at Austin