Trajectory Calculations for the Reaction of O Atoms with OH.

Abstract

Trajectory calculations have been used to calculate cross sections and specific rate constants for the two channels of the O + OH, reaction. Channel 1 is the exchange reaction O + O'H yields O' + OH, channel 2 the reaction O + OH yields H + OH2. From the specific rates, estimates of the overall thermal rate constants are calculated. The minimum thermal rate constant calculated for the channel 2 reaction is (5.4 + or - 0.7) x 10 to the -11th power cc/molecule sec. at 300 K, a value within error limits of that recommended by Wilson. The temperature dependence of this thermal rate constant, although higher, follows the shape of the curve of Kurzius and Boudart. The exchange reaction (channel 1) is estimated to be one third to one fifth as probable as the channel 2 reaction. (Author)

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1979
Accession Number
ADA069081

Entities

People

  • Arthur Gauss Jr.

Organizations

  • Ballistic Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Angular Momentum
  • Army Aviation
  • Atoms
  • Chemical Reactions
  • Chemistry
  • Combustion
  • Coordinate Systems
  • Energy
  • Exchange Reactions
  • Ground State
  • High Temperature
  • Integrators
  • Low Temperature
  • Molecules
  • Potential Energy
  • Quantum Chemistry
  • Trajectories

Readers

  • Combustion science or combustion engineering.
  • Molecular Photonics/Laser Physics