Dynamic and Static Stereochemistry in Dimolybdenum and Ditungsten Compounds Containing a Central (M Triple Bond M) +6 Unit.

Abstract

The chemistry of molybdenum and tungsten in oxidation state +3 is now dominated by compounds containing a central (M triple bond M) 6+ core, with metal-to-metal distances in the range of 2.2 to 2.3 A. The metal atoms may be bonded to three, four, five or six ligand atoms. Examples of each are given and for a given coordination number the preferred geometry is discussed. Low temperature nmr studies support the view that the structures found in the solid state are also present in solution. Variable temperature nmr studies reveal a wealth of knowledge concerning the dynamic behavior of those molecules in solution.

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Document Details

Document Type
Technical Report
Publication Date
Aug 29, 1979
Accession Number
ADA080467

Entities

People

  • Malcolm H. Chisholm

Organizations

  • Indiana University

Tags

Communities of Interest

  • Air Platforms
  • C4I

DTIC Thesaurus Topics

  • Chemical Bonds
  • Chemical Shifts
  • Chemical Synthesis
  • Chemistry
  • Geometry
  • Low Temperature
  • Magnetic Resonance
  • Metal Metal Bonds
  • Methylenes
  • Military Research
  • Molecular Orbital Theory
  • Nuclear Magnetic Resonance
  • Resonance
  • Stereochemistry
  • Transition Metals
  • Transitions
  • Universities

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry
  • Systems Analysis and Design