Synthesis and Properties of Acetylene Terminated Sulfone (ATS)

Abstract

The utilization of acetylene end-groups on phenylquinoxaline oligomers has provided a wide variety of new and improved matrix resins. The cured thermoset quinoxaline systems exhibit excellent moisture resistance which demonstrated the moisture insensitivity of the polyene product of the acetylene cure reaction. In an effort to use this technology in systems which process and handle like current state-of-the-art epoxies, the thermoset system 4,4'-bis(3- ethynylphenoxy)diphenylsulfone (ATS) was synthesized for characterization and evaluation as 350 deg F matrix system. Thermal analytical data obtained on ATS indicated a Tg at 0 deg C and a strong polymerization exotherm maximizing at 240 deg C. Cured ATS samples exhibited excellent thermal oxidative properties as evidenced by isothermal aging in air at 500 deg F and 600 deg F. Synthetic routes to ATS are included as well as physical properties of the system before/after cure.

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1980
Accession Number
ADA086148

Entities

People

  • F. E. Arnold
  • G. A. Loughran

Organizations

  • Wright Laboratory

Tags

Communities of Interest

  • Space

DTIC Thesaurus Topics

  • Acetylenes
  • Aeronautical Laboratories
  • Air Force
  • Air Force Facilities
  • Alkenes
  • Alkynes
  • Chemical Synthesis
  • Chemistry
  • Chlorides
  • Composite Materials
  • Infrared Spectra
  • Liquid Chromatography
  • Materials
  • Materials Laboratories
  • Moistureproofing
  • Resins
  • Thermal Properties

Fields of Study

  • Materials science

Readers

  • Polymer Science and Engineering.
  • Polymer Science and Technology