Amorphous-Crystalline Boundary Dynamics in Laser Crystallization.

Abstract

Two theoretical descriptions have been developed for the phase boundary dynamics during crystallization of amorphous films by scanning with the slit image of a cw laser or of any cw energy beam. The first reduces the problem to the solution of a one-dimensional integral equation, which allows a choice of initial conditions. Depending on the background temperature, numerical solutions yield either periodic or runaway motion of the amorphous-crystalline (a-c) boundary, as observed in experiments on scanned laser crystallization of thin films of a-Ge on fused-silica substrates. The calculations give a semi-quantitative fit to the experimental results for the spatial periodicity observed in the crystallized films as a function of background temperature. Profiles of film temperature as a function of distance from the laser image at successive times have been computed for both the periodic and runaway cases. The model qualitatively explains many of the effects observed during scanned cw laser crystallization, including periodic fluctuations in light emission. The second theoretical description is a more exact two-dimensional treatment, applicable only to cases of steady-state motion of the a-c boundary, which rigorously handles heat flow into the substrate. This treatment has been used to calculate the boundary velocity during steady-state runaway.

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Document Details

Document Type
Technical Report
Publication Date
Aug 25, 1981
Accession Number
ADA105811

Entities

People

  • Barbara J. Palm
  • Herbert J. Zeiger
  • John Chin C. Fan
  • Ralph L. Chapman
  • Ronald P. Gale

Organizations

  • Massachusetts Institute of Technology

Tags

Communities of Interest

  • Advanced Electronics
  • Air Platforms
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Critical Temperature
  • Crystal Structure
  • Crystallization
  • Energy
  • Equations
  • Films
  • Heat Energy
  • Heat Transmission
  • Integral Equations
  • Lasers
  • Latent Heat
  • Materials
  • Optical Materials
  • Phase Transformations
  • Steady State
  • Transition Temperature
  • Two Dimensional

Fields of Study

  • Physics

Readers

  • Calculus or Mathematical Analysis
  • Materials Science and Engineering.
  • Thermal Physics or Thermal Science.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition