Divalent Beta' Aluminas: High Conductivity Solid Electrolytes for Divalent Cations.

Abstract

The Na(+) content of beta alumina can be replaced by a variety of divalent cations in simple ion exchange reactions. The resulting divalent beta' aluminas are the first family of high conductivity solid electrolytes for first family of high conductivity solid electrolytes for divalent cations. Divalent beta' aluminas which have been prepared so far include conductors of Ca(2+), Sr(2+), Ba(2+), Zn(2+), Cd(2+), Pb(2+), Hg(2+), and Mn(2+). Most have conductivities of about 0.1/(ohm-cm) at 300-400 C. However, the conductivity of Pb(++) beta alumina is 0.0046/(ohm-cm) at 40 C, nearly equal to that of Na(+) beta alumina. Preliminary structure studies indicate that order-disorder reactions among the divalent cations and vacancies in the conduction region of beta alumina critically influence conductivity in the structure.

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Document Details

Document Type
Technical Report
Publication Date
Oct 13, 1982
Accession Number
ADA120675

Entities

People

  • B. Dunn
  • G. C. Farrington

Organizations

  • University of Pennsylvania

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Chemical Analysis
  • Chemistry
  • Crystal Lattices
  • Crystals
  • Electrolytes
  • Engineering
  • Exchange Reactions
  • Heat Of Activation
  • High Temperature
  • Ion Exchange
  • Materials
  • Materials Science
  • Measurement
  • Metals
  • Scattering
  • Single Crystals
  • Two Dimensional

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.