Investigation of Lithium Thionyl Chloride Battery Safety Hazards.

Abstract

Scanning electron and optical microscopic investigation of an overdischarged cathode from a cathode limited Li/SOCl2 cell reveal a three-dimensional reticulated lithium dendrite structure. Individual dendrites do not grow and longer than about 50 microns or any thicker than about 4 microns in diameter before branching at random angles. E.S.R. spectra of 50% and 100% overdischarged anode limited cells reveal a third chemical species carrying an unpaired electron which is distinct from the two radical species observed during discharge. No significant difference is observed between the Raman spectra of 100% discharged electrolyte and 50% cathode limited overdischarged electrolyte. The some holds true for infrared spectra. The Raman spectra of 90% anode limited overdischarged electrolyte shows most of the peaks occuring at 100% discharge in addition to 687, 727, 819, and 854 per cm. The infrared spectrum of the same solution shows most the the features occuring at 100% discharge in addition to the reduction of 981 cm-1 and growth of peaks at 1397,1085,1070 (shoulder) 661 and 602 cm-1. Peaks at 1070 and 661 always occur weakly in discharged electrolyte spectra and are quite strong in the spectrum of Li2S04 saturated electrolyte.

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Document Details

Document Type
Technical Report
Publication Date
Mar 31, 1982
Accession Number
ADA129300

Entities

People

  • Robert C. Mcdonald

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Chlorine
  • Electrochemical Reactions
  • Electrodes
  • Electrolytes
  • Electron Microscopes
  • Electron Spin Resonance
  • Filaments
  • Infrared Spectra
  • Lead Wires
  • Microscopes
  • Raman Spectra
  • Resonance
  • Scanning Electron Microscopes
  • Shoulder
  • Spectra
  • Spectroscopy
  • Spin Resonance

Fields of Study

  • Materials science

Readers

  • Battery Technology and Engineering
  • Materials Science and Engineering.
  • Mathematics or Statistics

Technology Areas

  • Microelectronics