The Chemical and Physical Properties of Pyrrole-Based Conducting Polymers: The Characterization of As-Grown Films by X-Ray Photoemission Spectroscopy.

Abstract

XPS techniques have been used to characterize electrically conducting films of polypyrrole and polybithiophenes grown electrochemically. These techniques have yielded information not only on the nature of the polymeric cation and its counter anion but also on the structural disorder in these polymers. In particular the N1s spectra have revealed a non-uniformity in the distribution of the anions relative to the nitrogen atoms and the C1s spectra clearly show that approximately 1/3 of the pyrrole rings are different from the rest. Significant improvement in the structural order is achieved by blocking the beta sites on the pyrrole ring with methyl groups to ensure a completely bonded polymer. Similar experiments on polybithiophene polymers show that this polymer is considerably more ordered than polypyrrole.

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Document Details

Document Type
Technical Report
Publication Date
Apr 07, 1983
Accession Number
ADA129486

Entities

People

  • G. B. Street
  • P. Pfluger

Organizations

  • International Business Machines Corporation (Armonk, NY)

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Band Spectra
  • Band Structures
  • Chemical Analysis
  • Chemistry
  • Conductive Polymers
  • Diseases And Disorders
  • Energy Bands
  • Fermi Levels
  • Films
  • Materials
  • Physical Properties
  • Polymeric Films
  • Polymers
  • Spectra
  • Spectroscopy
  • Valence Bands
  • X Rays

Fields of Study

  • Chemistry

Readers

  • Applied Combinatorial Optimization and Logic Circuit Design.
  • Polymer Science and Engineering.
  • Thin Film Deposition Science.