Nuclear Magnetic Relaxation in Polyacetylene.

Abstract

Nuclear spin-lattice relaxation rates for 1H and 13C in polyacetylene cannot be adequately explained in terms of either nuclear spin diffusion to a static paramagnetic defect or rapid one-dimensional diffusion of the defect itself. We propose a model in which only a small fraction of the molecular chains contain defects. Nuclei on these chains are rapidly relaxed, while the remainder achieve equilibrium by nuclear spin diffusion. The dependences of the measured relaxation rates upon frequency and isotopic concentration are in agreement with the predictions of this model.

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Document Details

Document Type
Technical Report
Publication Date
Apr 07, 1983
Accession Number
ADA129572

Entities

People

  • J. C. Scott
  • T. C. Clarke

Organizations

  • International Business Machines Corporation (Armonk, NY)

Tags

Communities of Interest

  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Conductive Polymers
  • Diffusion
  • Diffusion Coefficient
  • Domain Walls
  • Electron Spin Resonance
  • Electrons
  • Frequency
  • Low Temperature
  • Magnetic Resonance
  • Magnetization
  • Nuclear Spins
  • Nuclei
  • Quantum Properties
  • Recovery
  • Relaxation Time
  • Resonance
  • Spin Resonance

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Molecular Photonics/Laser Physics