Trace Chemical Threat Detection by Ultraviolet Multiphoton Induced Fragment Fluorescence

Abstract

ArF excimer laser radiation has been used to dissociate dimethylmethylphosphonate (DDMP) and diethylmethylphosphonothioate (DEMPS) into electronically excited fragments. Spectrally resolved UV and visible emission identifies the excited fragments from DMMP as C, C2 nd CH and those from DEMPS as C2, CH, PO and possibly PS and CS. In the few cases tested, the emission intensity is linear with respect to parent molecule concentration and persists in the presence of 100 torr of air. The excited fragment emissions could be the basis of a sensitive detection technique for these or similar molecules.

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1984
Accession Number
ADA140344

Entities

People

  • A. Freedman
  • C. E. Kolb
  • D. S. Frankel

Organizations

  • Aerodyne Research

Tags

Communities of Interest

  • C4I
  • Human Systems
  • Materials and Manufacturing Processes
  • Weapons Technologies

DTIC Thesaurus Topics

  • Absorption Coefficients
  • Biological Toxins
  • Chemical Warfare Agents
  • Chemical Weapons
  • Chemistry
  • Detection
  • Detectors
  • Excimer Lasers
  • Incapacitating Agents
  • Laser Beams
  • Laser Pulses
  • Lasers
  • Measurement
  • Organophosphorus Compounds
  • Phosgene
  • Quantum Yields
  • Scientists

Fields of Study

  • Physics

Readers

  • Analytical Chemistry
  • Quantum Chemistry
  • Spectroscopy.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Microelectronics