Kinetics of Simple Inner- and Outer-Sphere Electrochemical Reactions at Rotating Silver Electrodes as Examined Using Surface-Enhanced Raman Spectroscopy.

Abstract

An application of surface-enhanced Raman spectroscopy (SERS) to evaluating the kinetics of electrochemical reactions is outlined. This involves monitoring the potential-dependent SERS intensities of the adsorbed reactant at a rotating disk electrode in a potential region where the kinetics are under mixed mass transfer-heterogeneous electron transfer control. Comparisons are made between the kinetic behavior extracted from the SERS intensity-potential dependence and that obtained from the faradaic current flow.

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Document Details

Document Type
Technical Report
Publication Date
Sep 01, 1984
Accession Number
ADA145606

Entities

People

  • D. Milner
  • M. A. Tadayyoni
  • Michael J. Weaver
  • Stuart Farquharson

Organizations

  • Purdue University

Tags

Communities of Interest

  • Air Platforms

DTIC Thesaurus Topics

  • Chemical Reaction Properties
  • Chemistry
  • Current Density
  • Detectors
  • Electrochemical Reactions
  • Electrodes
  • Electron Transfer
  • Electrons
  • Kinetics
  • Mass Transfer
  • Raman Scattering
  • Raman Spectra
  • Raman Spectroscopy
  • Reaction Orders
  • Scattering
  • Spectra
  • Spectroscopy

Fields of Study

  • Chemistry

Readers

  • Computational Modeling and Simulation
  • Electrochemical Surface Science

Technology Areas

  • Microelectronics