Observation of a Novel Low-Lying Excited State in Zinc Complexes.

Abstract

A novel low-lying excited state(s) has been observed from emission studies of complexes of the type M(BS)2(S-phen) (M = Zn(II), Cd(II); BS = benzene thiol; s-phen = substituted 1,10-phenanthroline) at 77 K. The state is tentatively assigned to a charge-transfer configuration in which the thiol donates charge through the closed d-shell to the N-heterocyclic state geometry with respect to the ground state. The state decays on the order of microseconds, but its spin signature has not yet been determined. Originator furnished keywords include: excited states, emission, luminescence, charge transfer, zinc(II) complexes.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jan 22, 1985
Accession Number
ADA150188

Entities

People

  • G. A. Crosby
  • K. A. Truesdell

Organizations

  • Washington State University

Tags

Communities of Interest

  • Weapons Technologies

DTIC Thesaurus Topics

  • California
  • Charge Transfer
  • Chemistry
  • Civil Engineering
  • Emission
  • Emission Spectra
  • Engineering
  • Military Research
  • New Hampshire
  • Observation
  • Phosphorescence
  • Physics
  • Spectra
  • Technical Information Centers
  • United States
  • United States Government
  • Universities

Readers

  • Electrochemical Surface Science
  • Organic Chemistry
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.