The Electrochemistry of Azine, Oxazine and Thiazine Dyes

Abstract

The role of short-lived intermediates of dyes such as methylene blue safranin-O, neutral red and oxazines used in the photosensitization of electrodes was studied by means of laser flash photolysis and voltammetry. The study include transients initiated by absorption of light by dyes in solution and by dyes absorbed on electrodes, with major emphasis on the transients arising from solution absorption. For each mode of photoexcitation the identity, the lifetime and the mechanism of formation and decay of the transient species was determined. Key variables examined systematically included pH, solvent composition, electrode material and potential, and reagents which selectively quench the excited state. The goal established the place of formation and the disappearance of each transient species in the overall photoelectrochemical process.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 1985
Accession Number
ADA152394

Entities

People

  • David A. Aikens
  • Herbert H. Richtol

Organizations

  • Rensselaer Polytechnic Institute

Tags

DTIC Thesaurus Topics

  • Absorption
  • Chemical Compounds
  • Chemistry
  • Dyes
  • Electrochemical Cells
  • Electrochemistry
  • Electrodes
  • Indicator Dyes
  • Materials
  • Methylene Blue
  • Methylenes
  • Military Research
  • Photochemistry
  • Physical Chemistry
  • Redox Indicators
  • Specular Reflection
  • Voltammetry

Fields of Study

  • Chemistry

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Electrochemical Surface Science
  • Molecular Photonics/Laser Physics

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers