Re-Evaluation of Surface Properties of Oxide-Cathode Materials.

Abstract

Surface properties of high-surface-area samples of alkaline earth oxides BaO, MgO, SrO, and CaO - prepared singly as pure materials or as binary systems having BaO dispersed onto the surface of another of the oxides - have been examined using as probes the luminescence and the catalytic activity of the materials. Comparisons of results from the pure systems with those from the binary systems are consistent with extensive reconstruction (rumpling) of the surface layers of the surface-doped binary systems. Such rumpling can produce up to one half of a mono-layer of surface ions jutting out from the surface with a high degree of coordinative unsaturation and resultant high lability and catalytic activity.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jul 15, 1985
Accession Number
ADA161131

Entities

People

  • Joseph M Cunningham

Organizations

  • University College Cork

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Chemical Reactants
  • Chemical Reactions
  • Chemistry
  • Electron Microscopy
  • Electron Transfer
  • Emission Spectra
  • Energy Transfer
  • Isotopes
  • Mass Spectrometry
  • Measurement
  • Metal Oxides
  • Photoexcitation
  • Residuals
  • Spectrometry
  • Spectroscopy
  • Surface Properties
  • Transitions

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Materials Science and Engineering.
  • Surface Engineering/Surface Coating Technology.