An Experimental Evaluation of the Effects of Selected Organic Compounds on the Formation of Insolubles in Diesel Fuels.

Abstract

The study documents and interrelates five experimental programs conducted by the David Taylor Naval Ship Research and Development Center in-house and under contract. The programs were designed to increase understanding of the effects of eleven selected heterocompounds on the stability of diesel-range fuels. The programs employed any or all of four different stability tests ranging from an oven test conducted at 150 F (65.6) for periods up to eight weeks to a test which exposed the fuel to a temperature of 500 F (260 C) for a few seconds. Ranking of the fuels and fuel mixes by all of the tests was reasonably consistent. The nature of the base fuel was important in determining the amount of sediment formed in the presence of a given heterocompound. Of the nine compounds individually tested, 2,5-dimethylpyrrole (DMP) and 1,2,5-trimethylpyrrole produced the greatest amounts of sediment, and 2- methylpiperazine (MPPZ), 1-dodecanethiol (DDSH), and 2,6-di-tert-butylphenol the least. Also, DDSH over a range of concentrations showed a synergistic effect in the presence of a constant level of DMP. In a synergistic effect in the presence of a constant level of DMP. In contrast, MPPZ inhibited the formation of sediment in the presence of an equivalent concentration of DMP. A number of sediment mass versus time curves gave evidence of an inducation period. Curves of sediment mass versus compound concentration was roughly linear. Originator supplied keywords include: Storage stability; Thermal stability; Oxidative stability; Oxygen compounds; Gum formation rates; Sediment formation rates; Nitrogen compounds; Heterocompounds; Sulfur compounds.

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Document Details

Document Type
Technical Report
Publication Date
Nov 01, 1985
Accession Number
ADA161323

Entities

People

  • John G. Zimmerman

Tags

Communities of Interest

  • Air Platforms
  • Ground and Sea Platforms

DTIC Thesaurus Topics

  • Chemical Synthesis
  • Chemistry
  • Diesel Fuels
  • High Temperature
  • Jet Engine Fuels
  • Materials Laboratories
  • Materials Science
  • Materials Testing
  • New York
  • Nitrogen Compounds
  • Organic Compounds
  • Oxygen Compounds
  • Petroleum
  • Plastic Explosives
  • Rate Of Formation
  • Test Methods
  • United States Naval Academy

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  • Analytical Chemistry
  • Mathematics or Statistics
  • Petroleum Engineering