The Molecular Structures of Cis- and Trans-1, 2-Dichloroethene: A Real-Time Gas Electron Diffraction and AG Initio Study,

Abstract

The molecular structures of cis- aand trans-1,2-dichloroethene were studied in the gas phase by electron diffraction, using our new real-time data acquisition technique. For cis-dichloroethene the structural parameters are (r sub a distances (Angstroms) and angles (deg), with 3sigma in parentheses): C-C1:1.717(2); C=C:1.337(4); C1-C=C: 124.0(2); and H-C=C:120.3(3). For trans-dichloroethene: C-C1:1.725(2); C=C:1.332(8); C1-C=C:120.8(6); and H-C=C:124.0(3). The experimental work was augmented by ab initio gradient geometry refinements of the two compounds and of cis- and trans-difluorothene. The 4-21G, 5-31G**, and 3-3-21G basis sets were used in various series of calculations. Without any exception, the calculated structural trends for the cis- and trans-configurations are in excellent agreement with the experiments.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 1985
Accession Number
ADA169617

Entities

People

  • David L. Monts
  • David W. Paul
  • John D. Ewbank
  • Khamis Siam
  • Lothar Shafer

Organizations

  • University of Arkansas

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  • Energy and Power Technologies

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  • Acquisition
  • Agreements
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  • Amplitude
  • Arkansas
  • Chemical Compounds
  • Chemistry
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  • Data Acquisition
  • Diffraction
  • Distribution Curves
  • Electron Diffraction
  • Electrons
  • First Principles Calculations
  • Intensity
  • Molecular Structure
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  • Chemistry

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