Studies of Chain Conformational Kinetics in Poly(Di-n-Akylsilanes) by Spectroscopic Methods. 2. Conformation and Packing of Poly(Di-n-Hexylsilane),

Abstract

Unoriented and highly oriented films of poly(di-n-hexylsilane) have been studied by Raman scattering, wide angle X-ray diffraction and optical absorption measurements. From a comparison of group theoretical predictions with those bands observed in the Raman experiments and from the X-ray layer line spacing in an oriented sample, a planar zig-zag conformation for the silicon backbone was deduced. X-ray reflections were suitable indexed by a monoclinic unit cell containing two molecules. Polarized Raman studies on uniaxiallly oriented samples also revealed that the hexyl side chains are not orthogonal to the silicon backbone but may be slightly titled in order to minimize intramolecular steric interactions.

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Document Details

Document Type
Technical Report
Publication Date
Aug 07, 1986
Accession Number
ADA170690

Entities

People

  • B. L. Farmer
  • H. Kuzmany
  • J. F. Rabolt
  • R. D. Miller

Organizations

  • International Business Machines Corporation (Armonk, NY)

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Diffraction
  • Diffractometers
  • Frequency
  • Frequency Bands
  • Frequency Shift
  • Materials
  • Materials Science
  • Measurement
  • Molecules
  • Phase Transformations
  • Raman Scattering
  • Raman Spectra
  • Scattering
  • Spectra
  • Transition Temperature
  • Transitions
  • Wide Angles

Fields of Study

  • Chemistry

Readers

  • Materials Science and Engineering.
  • Polymer Science and Technology

Technology Areas

  • Space