Photodissociation of Gaseous Ions Formed by Laser Desorption.

Abstract

Both pulsed and gated continuous wave carbon dioxide lasers have been employed to desorb ions and then to photodissociate them in a Fourier transform ion cyclotron resonance mass spectrometer. Pulsed CO2 laser irradation was most successful in laser desorption experiments, while a gated continuous wave laser was used for a majority of the successful infrared multiphoton dissociation studies. Fragmentation of ions with m/z values in the range 400-1300 was induced by infrared multiphoton dissocation. Such photodissociation was successfully coupled with laser desorption for a number of different classes of compounds. Either two sequential pulses from a pulsed carbon dioxide laser (one for desorption and one for dissociation) or one desorption pulse followed by gated continuous wave irradation to bring about dissociation were ultilized. Keywords: Carbon Dioxide Lasers; Fourier Transform; Ion Cyclotron Resonance; Mass Spectrometry; Infrared Multiphoton Dissociation; Laser Desorption.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Sep 20, 1986
Accession Number
ADA172621

Entities

People

  • Clifford H. Watson
  • Gokhan Baykut
  • John R. Eyler

Organizations

  • University of Florida

Tags

Communities of Interest

  • Advanced Electronics
  • Weapons Technologies

DTIC Thesaurus Topics

  • Abstracts
  • Carbon Dioxide
  • Carbon Dioxide Lasers
  • Chemical Synthesis
  • Chemistry
  • Continuous Waves
  • Cyclotron Resonance
  • Dye Lasers
  • Infrared Lasers
  • Laser Beams
  • Lasers
  • Mass Spectra
  • Mass Spectrometers
  • Mass Spectrometry
  • Military Research
  • Spectrometry
  • Standards

Fields of Study

  • Physics

Readers

  • Molecular Photonics/Laser Physics

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers