Environmental Fate of White Phosphorus/Felt and Red Phosphorus/Butyl Rubber Military Screening Smokes

Abstract

Investigations were conducted to identify those processes that control the loss and movement of White phosphorus/felt, Red phosphorus/butyl rubber, and their combustion products in air, soil, and aquatic environments. The fate of RP/BR will be controlled by oxidative transformation. In air, half- lives of 1.8 years were found while in aerated water, the half-life approach 3 years and was found to be dependent on both particle size and oxygen concentration. In soil, the transformation was limited by oxygen diffusion and half-lives into the thousands of years were projected. The oxidative transformation and combustion of WP/F and RP/BR lead to the formation of linear condensed polyphosphates, (P10P22), phosphoric acid, phosphorous acid, hypophosphorous acid, and phosphine. The linear polyphosphates hydrolyze rapidly at low pH (t1/2 = 2 days) which is expected in the aerosol phase. In a neutralized state, the polyphosphates are subject to slow chemical hydrolysis (t1/2 = 100 days). Microorganisms will hydrolyze linear polyphosphates in soils and water with half lives of 15 days in systems containing 100,000 organisms/ml (gm). Cyclic meta-phosphates (tri-, tetra-, and (hexa-) are formed from the linear polyphosphates in aqueous solution and are stable to chemical hydrolysis (t1/2 = 3 years). However, microorganisms can utilize these compounds as a phosphate source with a half-life of 20 days.

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Document Details

Document Type
Technical Report
Publication Date
Apr 01, 1985
Accession Number
ADA176922

Entities

People

  • R. T. Podoll
  • Robert Rewick
  • Robert Wilson
  • Ronald J. Spanggord
  • Tsong-wen Chou

Organizations

  • SRI International

Tags

Communities of Interest

  • Biomedical
  • Weapons Technologies

DTIC Thesaurus Topics

  • Aqueous Solutions
  • Chemical Products
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Combustion
  • Combustion Products
  • Computers
  • Environment
  • Heat Of Solution
  • Microorganisms
  • Partial Pressure
  • Particle Size
  • Physical Properties
  • Rate Of Formation
  • Vapor Pressure

Readers

  • Agricultural Chemistry/Soil Science
  • Analytical Chemistry
  • Toxicology/Environmental Toxicology