Pressure Studies of Protein Dynamics.

Abstract

The relation between dynamic structure and function of proteins is investigated. Protein dynamics are studied by observing the phenomena induced by flash photolysis using near ultraviolet, optical, and infrared spectroscopies over wide ranges in temperature (60-300 K), time (50ns-lks), and, most importantly for this grant, pressure (0.1-200MPA). A simple biomolecular reaction - carbon monoxide binding to myoglobin is studied. Previous work over wide ranges in temperature and time has been crucial to developing models of protein dynamics. Pressure effects are less well explored. Studies over wide ranges of both temperature and pressure can probe protein states which are not accessible by varying only temperature or pressure. A hierarchical model of protein dynamics was developed which promises to contribute to understanding both biomolecular reactions and the physics of amorphous solids and glasses. The combined pressure and temperature experiments will test various features of the hierarchical model including the glass-like properties of proteins. keywords: myoglobin.

Document Details

Document Type
Technical Report
Publication Date
Feb 28, 1987
Accession Number
ADA177825

Entities

People

  • Hans Frauenfelder
  • Robert D. Young

Organizations

  • University of Illinois Urbana–Champaign

Tags

DTIC Thesaurus Topics

  • Amorphous Materials
  • Carbon Monoxide
  • Dielectric Gases
  • Dynamics
  • Infrared Spectroscopy
  • Materials
  • Monoxides
  • Photolysis
  • Physics
  • Spectroscopy

Readers

  • Computational Fluid Dynamics (CFD)
  • Molecular Photonics/Laser Physics
  • Molecular and Cellular Biochemistry