Electron Paramagnetic Resonance on Asphaltic Materials

Abstract

Asphalts have been used as paving materials for many years and a great deal of research has been conducted in the physical properties needed for good for good performance. In the past, some chemical research has been performed on these materials as well. Questions have remained as to what chemical properties are important in the design of a long-lasting pavement structure. This study has used a spectroscopic technique to investigate the aging and catalytic properties of asphalts. Electron Paramagnetic Resonance (EPR) was used to identify the role of free-radical species in these processes. Two paramagnetic categories were identified: organic free radicals and vanadium transition metal ions. Free radical and transition metals are highly reactive, and may play important roles in the oxidation process that contributes to aging. The results of this study indicate that there may be a relationship between the concentrations of the free radical species to the aging index and to the changes in the specific clay gel fractions. Keywords: Asphalt; spectroscopic technique; vanadium ions; transition metal.

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 1987
Accession Number
ADA178471

Entities

People

  • Betty J. Humphrey

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies
  • Human Systems

DTIC Thesaurus Topics

  • Air Force
  • Air Force Facilities
  • Chemical Properties
  • Chemical Synthesis
  • Chemistry
  • Chlorides
  • Electron Paramagnetic Resonance
  • Elements
  • Magnetic Fields
  • Organic Chemistry
  • Paramagnetic Resonance
  • Physical Properties
  • Resonance
  • Spectra
  • Spectroscopy
  • Standards
  • Transition Metals

Readers

  • Organic Chemistry
  • Pavement Materials Engineering.
  • Theoretical Analysis.

Technology Areas

  • Microelectronics