Emission Spectroscopic Evidence of Bronsted Acid Sites in a Calcinated Vycor Glass.
Abstract
The emission and excitation spectra of quinoline and 2,3-dichloroquinozaline embedded in a calcinated (600 C) porous Vycor glass and dissolved in fluid solutions were recorded at various temperatures. The spectral characteristics and phosphorescence lifetimes of adsorbates were observed to be identical to those in 0.5 N sulphonic acid solutions, indicating that H+ transferred from the surface to the N-heterocyclics. The strong surface-adsorbate interaction is further revealed by the dynamic study of adsorbates at 77 and 4.2K.
Document Details
- Document Type
- Technical Report
- Publication Date
- May 18, 1987
- Accession Number
- ADA181120
Entities
People
- C. L. Yang
- C. T. Lin
- Mostafa El-Sayed
- W. L. Hsu
Organizations
- University of California, Los Angeles