Laser Induced Surface Chemical Epitaxy: A Novel Thin Film Deposition Technique.

Abstract

This report identifies a new deposition technique, laser induced surface chemical epitaxy, and describes experimental studies of the surface chemistry relevant to the feasibility of the technique. The experiments focus on the thermal and photo-induced surface chemistry of two organometallic molecules, dimethyl cadmium and dimethyl tellurium, on a variety of surfaces including GaAs, Au, Si, and SiO2. These studies followed ultra-high vacuum compatible procedures and used x-ray photoelectron spectroscopy to characterize thermal and photon-induced effects on the chemical state of the adsorbed organometallic molecule. The results show considerable diversity in the thermal surface chemistry of the system investigated. Physisorption and dissociative chemisorption to yield monomethyl and metal adspecies were observed. Irradiation of the physisorbed adspecies with 193 nm UV photons caused both photodecompositon and photodesorption. Similar irradiation of the photons caused both photodecomposition and photodesorption. Keywords: Lasers; Epitaxy; Thin films; Deposition; Surface chemistry.

Document Details

Document Type
Technical Report
Publication Date
Apr 15, 1987
Accession Number
ADA181216

Entities

People

  • Andrew Freedman
  • Charter D. Stinespring

Organizations

  • Aerodyne Research

Tags

DTIC Thesaurus Topics

  • Chemisorption
  • Chemistry
  • Films
  • High Vacuum
  • Molecules
  • Photodecomposition
  • Photoelectrons
  • Spectroscopy
  • Surface Chemistry
  • Tellurium
  • Thin Films
  • Vacuum
  • X Ray Photoelectron Spectroscopy
  • X Rays

Fields of Study

  • Materials science

Readers

  • Molecular Photonics/Laser Physics
  • Thin Film Deposition Science.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition
  • Microelectronics
  • Microelectronics - Graphene