Re-Usable Thin-Layer Spectroelectrochemical Cell for Non-Aqueous Solvent Systems.

Abstract

A thin layer spectroelectrochemical cell for use with aqueous or organic solvent systems is described and evaluated. The cell design, comprising a working chamber formed by sandwiching Teflon spacers between two optical windows and a Teflon body, allows versatility of the working electrode material, and is easily dismantled and reassembled. Variation of the window material permits measurements to be made over a wide spectroscopic range, from the uv visible to the infrared regions. The performance of the cell is assessed for a gold minigrid working electrode in the uv-visible region using the oxidation of 2,9,16,23-tetra(neopentoxy)-phthalocyaninato zinc to its pi-cation radical in o-dichlorobenzene, and in the infrared region by investigating the reductions of bis(2,2'-bipyridine)(2,2'-azodpyridine)ruthenium(II) bis(hexafluorophosphate) in deuterated dimenthylsulfoxide.

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Document Details

Document Type
Technical Report
Publication Date
Nov 01, 1987
Accession Number
ADA186951

Entities

People

  • Alfred Beverley Philip Lever
  • W. A. Nevin

Organizations

  • University of York

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Abstracts
  • Acquisition
  • Air Force
  • Aqueous Solutions
  • Assembly
  • Chemical Compounds
  • Chemical Engineering
  • Chemical Synthesis
  • Chemistry
  • Electrodes
  • Engineering
  • Materials
  • Materials Science
  • Military Research
  • New York
  • Physics
  • United States

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  • Electrical Engineering
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Electrochemical Surface Science